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Double Rabi Splitting in a Strongly Coupled System of Core-Shell Au@Ag Nanorods and J-Aggregates of Multiple Fluorophores

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dc.contributor.authorMelnikau, D.
dc.contributor.authorGovyadinov, A. A.
dc.contributor.authorSanchez-Iglesias, A.
dc.contributor.authorGrzelczak, M.
dc.contributor.authorNabiev, I. R.
dc.contributor.authorLiz-Marzan, L. M.
dc.contributor.authorRakovich, Y. P.
dc.contributor.authorНабиев, Игорь Руфаилович
dc.date.accessioned2024-11-21T12:26:33Z
dc.date.available2024-11-21T12:26:33Z
dc.date.issued2019
dc.description.abstractCopyright © 2019 American Chemical Society.The interaction of several components in the strong coupling regime yielding multiple Rabi splittings opens up remarkable possibilities for studies of multimode hybridization and energy transfer, which is of considerable interest in both fundamental and applied science. Here we demonstrate that three different components, such as core-shell Au@Ag nanorods and J-aggregates of two different dyes, can be integrated into a single hybrid structure, which leads to strong collective exciton-plasmon coupling and double-mode Rabi splitting totaling 338 meV. We demonstrate strong coupling in these multicomponent plexitonic nanostructures by means of magnetic circular dichroism spectroscopy and demonstrate strong magneto-optical activity for the three hybridized states resulting from this coupling. The J-aggregates of two different nonmagnetic dyes interact with metal nanoparticles effectively, achieving magnetic properties due to the hybridization of electronic excitations in the three-component system. ©
dc.format.extentС. 6137-6143
dc.identifier.citationDouble Rabi Splitting in a Strongly Coupled System of Core-Shell Au@Ag Nanorods and J-Aggregates of Multiple Fluorophores / Melnikau, D. [et al.] // Journal of Physical Chemistry Letters. - 2019. - 10. - № 20. - P. 6137-6143. - 10.1021/acs.jpclett.9b01988
dc.identifier.doi10.1021/acs.jpclett.9b01988
dc.identifier.urihttps://www.doi.org/10.1021/acs.jpclett.9b01988
dc.identifier.urihttps://www.scopus.com/record/display.uri?eid=2-s2.0-85073001837&origin=resultslist
dc.identifier.urihttp://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=Alerting&SrcApp=Alerting&DestApp=WOS_CPL&DestLinkType=FullRecord&UT=WOS:000492425100024
dc.identifier.urihttps://openrepository.mephi.ru/handle/123456789/18752
dc.relation.ispartofJournal of Physical Chemistry Letters
dc.titleDouble Rabi Splitting in a Strongly Coupled System of Core-Shell Au@Ag Nanorods and J-Aggregates of Multiple Fluorophores
dc.typeArticle
dspace.entity.typePublication
oaire.citation.issue20
oaire.citation.volume10
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relation.isAuthorOfPublication.latestForDiscoverya4923e3c-317e-498d-a747-cad6d3054e23
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