Персона: Савченков, Павел Сергеевич
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Induced magnetism and “magnetic hole” in singlet ground state system PrNi
© 2019 Elsevier B.V.The phenomenon of “induced magnetic ordering” for the local magnetic moments with singlet ground state in a periodical lattice is considered for the prototype intermetallic rare-earth compound PrNi ordered ferromagnetically at temperature TC = 21 K. Within the framework of a realistic model the energy dispersion relations are obtained for the magnetic excitations above Tc along the high symmetry directions. The “soft mode” behaviour observed for the acoustic magnetic excitation along (q 0 0) direction is reproduced. The influence of the substitution of isovalent nonmagnetic La for Pr1−xLaxNi on the temperature of ferromagnetic ordering is investigated. The linear decrease of the ordering temperature TC down to zero value in increasing of the La concentration up to x = 0.5 is observed and described by the model.
Neutron magnetic form factor in studies of f-electron instability
Multimodal reconstruction of TbCo thin-film structure with Bayesian analysis of polarized neutron reflectivity
Experimental Setup for Methodological Research with Polarized Neutrons at the IR-8 Reactor
Dramatic impact of intermediate-valence impurity on induced magnetism in singlet ground state system PrNi
© 2020 Elsevier B.V.We studied the influence of La (nonmagnetic) and Ce (intermediate valence) impurities on the ferromagnetic ordering temperature Tc of compounds RE1-x(La,Ce)xNi (RE = Pr, Gd). The ordering temperature Tc was measured in a wide range of impurity concentration. Crystal electric field (CEF) splitting for the PrNi and Pr0.25Ce0.75Ni was defined by neutron spectroscopy measurements. The strong difference in the influence of La and Ce on Tc of PrNi and GdNi based systems has been obtained. The introduction of a spin-fluctuating intermediate valence impurity in PrNi leads to a dramatic increase in the area of the ordered state on the phase diagram, due to an increase in Tc, compared to the impact of La-impurity over the entire concentration range. The dependence of Tc on the Ce concentration for the Pr1-xCexNi was calculated within the framework of the model of microscopic states. The essential modification of the CEF splitting by the Ce impurity appears to be the decisive factor affecting Tc wherein the Ce ion carries zero static magnetic moments similar to the La case. The latter explains the identical dependencies of the ordering temperature on the impurity concentration observed in systems with a long-range order of local magnetic moments Gd1-xLaxNi and Gd1-xCexNi.