Персона: Лебединский, Юрий Юрьевич
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Институт лазерных и плазменных технологий
Стратегическая цель Института ЛаПлаз – стать ведущей научной школой и ядром развития инноваций по лазерным, плазменным, радиационным и ускорительным технологиям, с уникальными образовательными программами, востребованными на российском и мировом рынке образовательных услуг.
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Юрий Юрьевич
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- ПубликацияТолько метаданныеA Unique System for Registering One-Photon Signals in the Ultraviolet Range from An Isomeric 229mTh Nucleus Implanted on Thin SiO2/Si Films(2020) Lebedinskii, Y. Y.; Borisyuk, P. V.; Chubunova, E. V.; Kolachevsky, N. N.; Vasiliev, O. S.; Tkalya, E. V.; Лебединский, Юрий Юрьевич; Борисюк, Петр Викторович; Чубунова, Елена Витальевна; Васильев, Олег Станиславович; Ткаля, Евгений Викторович© 2019 WILEY-VCH Verlag GmbH & Co. KGaA, WeinheimCurrently, an urgent task related to creating a nuclear frequency standard is the identification of a low-lying nuclear state in the thorium-229 isotope. Herein, a method for measuring the single-photon energy during the decay of an isomeric thorium-229 nucleus implanted in a wide-gap dielectric SiO2 (Eg = 9 eV) is developed. The proposed method utilizes thin silicon oxide layers obtained by thermal oxidization of the pure silica wafers, which allows measurement of the energy of photons in the ultraviolet (UV) range using an electronic spectrometer. The modeling study of electronic state excitation is provided via UV radiation from Kr, Xe, and D resonance discharging lamps. The obtained spectra are analyzed, and a method for determining the UV photon's energy is proposed.
- ПубликацияТолько метаданныеFormation and properties of thin Mo and Mo oxide nanoparticle films(2020) Borisyuk, P. V.; Vasilyev, O. S.; Lebedinskii, Y. Y.; Bortko, D. V.; Balakhnev, K. M.; Борисюк, Петр Викторович; Васильев, Олег Станиславович; Лебединский, Юрий Юрьевич; Бортко, Диана Владимировна; Балахнёв, Кирилл Максимович© 2019 Elsevier B.V.The paper presents a study of thin Mo films, consisted of individual nanoparticles of 3.5–5.5 nm in diameter. Their chemical, electron, and optical properties are studied. It is shown that thin films consisting of individual Mo nanoparticles can be formed from the gas phase by magnetron sputtering. Atmospheric exposure leads to the formation of MoOx oxide shell around the metal nuclei of Mo nanoparticles in the films and changes in its electronic structure. Optical properties of the obtained films consisted of ‘core–shell’ Mo@MoOx nanoparticles are investigated. It is shown that the absorption window falls on the range of 190–300 nm, which can be used in the development of single-photon detectors sensitive to weak ultraviolet signals from long-live states, for example from Th-229 low-lying isomeric state.
- ПубликацияТолько метаданныеFormation of Thin-Film Nanoparticle Materials for Single-Photon Avalanche Detectors(2020) Vasilyev, O. S.; Borisyuk, P. V.; Lebedinskii, Y. Y.; Васильев, Олег Станиславович; Борисюк, Петр Викторович; Лебединский, Юрий Юрьевич© 2020, Pleiades Publishing, Ltd.Abstract: The results of the formation of an original material based on thin films of metal nanoclusters and the investigation of its chemical composition, surface morphology, and structure are presented. Monodisperse thin films comprised of individual nanoclusters of Ta, Mo, and Ni metals were manufactured by gas-phase magnetron sputtering. Images of the surface were obtained by scanning electron microscopy and it was shown that the Ta and Mo films had a well-developed porous structure and consisted of separate nanoclusters contacting each other only at the interface. The chemical composition of the resulting films immediately after deposition (in situ) and after exposure to the atmosphere (ex situ) was investigated by X-ray photoelectron spectroscopy. It was shown that the exposure to the atmosphere led to the oxidation of the obtained films, namely, to the formation of oxide shells in nanoclusters that formed the films. The possibility of creating thin-film photodetectors based on nanocluster films to detect the decay of isomeric nuclear transition in 229Th nuclei is discussed.
- ПубликацияТолько метаданныеThSi10O22 Compound as Target for Production of Isomeric Thorium-229 Nuclei at Electron Beam Irradiation(2020) Borisyuk, P. V.; Chubunova, E. V.; Lebedinskii, Y. Y.; Vasilyev, O. S.; Yakovlev, V. P.; Борисюк, Петр Викторович; Чубунова, Елена Витальевна; Лебединский, Юрий Юрьевич; Васильев, Олег Станиславович; Яковлев, Валерий Петрович© 2020, Pleiades Publishing, Ltd.Abstract: A method for excitation of thorium-229 isomeric nuclei the electron beam irradiation of a solid-state target based on thorium silicate is considered. The key point for obtaining an effective yield of isomeric nuclei is the generation of secondary electrons with a significant increase in the multiplication factor for electrons that have energies within a range from 1 to 25 keV. Based on numerical simulation and theoretical estimation of the excitation cross section of isomeric transition in inelastic scattering, the yield function of isomeric nuclei was o qualitatively obtained.
- ПубликацияТолько метаданныеThe Electronic and Optical Properties of Thin Nanocluster Mo Films for Single-Photon UV Detectors(2020) Vasilyev, O. S.; Borisyuk, P. V.; Lebedinskii, Y. Y.; Васильев, Олег Станиславович; Борисюк, Петр Викторович; Лебединский, Юрий Юрьевич© 2020, Pleiades Publishing, Ltd.Abstract: Results of a study of the electronic structure and optical properties of a novel material based on thin films comprised of Mo nanoclusters obtained by gas-phase magnetron sputtering are presented. The chemical composition of the obtained films immediately after deposition (in situ) and upon exposure to the atmosphere (ex situ) was investigated by X-ray photoelectron spectroscopy. It is shown that exposure to the atmosphere leads to “core–shell” oxidation of the nanoclusters the obtained films are composed of and changes in the valence band. The change in the electronic structure of the obtained films was investigated by spectro-scopy of the characteristic energy losses of electrons. The optical properties of the obtained films were investigated in the wavelength range of 185–800 nm. The possibility of creating thin-film photodetectors based on the obtained Mo nanocluster films for detecting isomeric nuclear transition decay in 229Th nuclei is discussed.
- ПубликацияТолько метаданныеThin Ta/Ta oxide core-shell nanoparticle film size-dependent energy structure(2021) Borisyuk, P. V.; Vasilyev, O. S.; Lebedinskii, Y. Y.; Bortko, D. V.; Karazhanov, S.; Борисюк, Петр Викторович; Васильев, Олег Станиславович; Лебединский, Юрий Юрьевич; Бортко, Диана Владимировна; Каражанов, Смагул Жангабергенович© 2020 Elsevier B.V.The paper presents the research of thin films, consisting of spherical monodisperse Ta particles. For different samples particle sizes varied from 1.3 nm to 5.8 nm. The films were also exposed to the atmosphere for oxidation, which resulted in formation of a core-shell particle structure, where core was metal and shell was Ta oxide (Ta2O5). Dependency of bandgap Egap and valence band offset (VBO) on particle size has been investigated for the structure by using the X-ray photoelectron spectroscopy (XPS) and reflected electron energy loss spectroscopy (REELS) methods. We have found, that Egap decreases from 4.72 eV to 4.47 eV whereas VBO decreases from 3.50 eV to 2.95 eV with increasing the particle size. A new method of a fine regulation of the electronic structure is suggested, particularly for the application in ultraviolet (UV) photodetector design for low-lying nuclear and electron transitions detection.
- ПубликацияТолько метаданныеAutoelectronic emission and charge relaxation of thorium ions implanted into a thin-film silicon oxide matrix(2021) Borisyuk, P. V.; Chubunova, E. V.; Kolachevsky, N. N.; Lebedinskii, Y. Y.; Tkalya, E. V.; Vasilyev, O. S.; Yakovlev, V. P.; Борисюк, Петр Викторович; Чубунова, Елена Витальевна; Лебединский, Юрий Юрьевич; Ткаля, Евгений Викторович; Васильев, Олег Станиславович; Яковлев, Валерий ПетровичAn ensemble of thorium-229 ions embedded by pulsed laser implantation into a matrix of a broadband dielectric-silicon oxide is studied. The results of the experimental investigation of thorium ions' lifetime as charged components of the Th+/SiO2/Si system formed immediately after laser implantation are presented. The modelled theoretical description takes into account the instantaneous charging of the surface via laser implantation followed by charge relaxation due to the effect of autoelectronic emission that leads to time dependent partial neutralization of the surface charge by tunneling electrons. It was found that the lifetime of Th+ ions on the SiO2 surface can exceed 10 s, which would be an attractive opportunity for studying the nuclear low-lying isomeric transition in the thorium-229 isotope.